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The following table gives some reactivity ratios for various comonomer pairs. Fo

ID: 482759 • Letter: T

Question

The following table gives some reactivity ratios for various comonomer pairs. For each pair, calculate:

a) the composition of the copolymer formed at low conversions of an equimolar mixture of the two monomers. Show an example calculation. Note: I have given you the answer to the first pair so that you can check your approach.

b) the comonomer composition required to form a copolymer consisting of 50 mol.% styrene repeat units. Show an example calculation. Note: I have given you the answer to the first pair so that you can check your approach.

Monomer 1 Monomer 2 Equimolar Composition ri composition or 50 mol% styrene (b Styrene Butadiene 0.78 1.39 42.7 mol 57.2 mol Styrene Styrene 0.52 046 Styrene Methyl methacrylate Styrene Acrylonitrile 0.40 0.04 Styrene Vinyl chloride 17 0.02 Description

Explanation / Answer

F1 = [r1 f12 + f1 f2] / [r1 f12 + 2 f1 f2 + r2 f22]

where F1 = Mole fraction of monomer 1 in copolymer

f1 = Mole fraction of monomer 1 in feed = 0.5 (as equimolar composition)

f2 = Mole fraction of monomer 2 in feed = 0.5 (as equimolar composition)

r1 = Reactivity ratio of monomer 1

r2 = Reactivity ratio of monomer 2

1. Styrene and Butadiene

r1 = 0.78, r2 = 1.39

F1 = [r1 f12 + f1 f2] / [r1 f12 + 2 f1 f2 + r2 f22]

= [(0.78) (0.5)2 + (0.5) (0.5)] / [(0.78) (0.5)2 + (2) (0.5) (0.5) + (1.39) (0.5)2]

= 0.445 / 1.0425 = 0.427 = 0.427 x 100 = 42.7%

Equimolar composition = 42.7%

2. Styrene and Methyl methacrylate

r1 = 0.52, r2 = 0.46

F1 = [r1 f12 + f1 f2] / [r1 f12 + 2 f1 f2 + r2 f22]

= [(0.52) (0.5)2 + (0.5) (0.5)] / [(0.52) (0.5)2 + (2) (0.5) (0.5) + (0.46) (0.5)2]

= 0.38 / 0.745 = 0.510 = 0.510 x 100 = 51.0%

Equimolar composition = 51.0%

3. Styrene and Acrylonitrile

r1 = 0.40, r2 = 0.04

F1 = [r1 f12 + f1 f2] / [r1 f12 + 2 f1 f2 + r2 f22]

= [(0.40) (0.5)2 + (0.5) (0.5)] / [(0.40) (0.5)2 + (2) (0.5) (0.5) + (0.04) (0.5)2]

= 0.35 / 0.61 = 0.574 = 0.574 x 100 = 57.4%

Equimolar composition = 57.4%

4. Styrene and Vinyl chloride

r1 = 17, r2 = 0.02

F1 = [r1 f12 + f1 f2] / [r1 f12 + 2 f1 f2 + r2 f22]

= [(17) (0.5)2 + (0.5) (0.5)] / [(17) (0.5)2 + (2) (0.5) (0.5) + (0.02) (0.5)2]

= 4.50 / 4.755 = 0.946 = 0.946 x 100 = 94.6%

Equimolar composition = 94.6%

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